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dc.contributor.authorBachellier, N.
dc.contributor.authorVerlhac, B.
dc.contributor.authorGarnier, L.
dc.contributor.authorZaldívar, J.
dc.contributor.authorRubio Verdú, Carmen
dc.contributor.authorAbufager, P.
dc.contributor.authorOrmaza, M.
dc.contributor.authorChoi, D. J.
dc.contributor.authorBocquet, M. L.
dc.contributor.authorPascual Chico, José Ignacio ORCID
dc.contributor.authorLorente Palacios, Nicolás
dc.contributor.authorLimot, L.
dc.date.accessioned2020-04-21T08:58:44Z
dc.date.available2020-04-21T08:58:44Z
dc.date.issued2020-04
dc.identifier.citationNature Communications 11 : (2020) // Article ID 1619es_ES
dc.identifier.issn2041-1723
dc.identifier.urihttp://hdl.handle.net/10810/42835
dc.description.abstractThe electrical control and readout of molecular spin states are key for high-density storage. Expectations are that electrically-driven spin and vibrational excitations in a molecule should give rise to new conductance features in the presence of magnetic anisotropy, offering alternative routes to study and, ultimately, manipulate molecular magnetism. Here, we use inelastic electron tunneling spectroscopy to promote and detect the excited spin states of a prototypical molecule with magnetic anisotropy. We demonstrate the existence of a vibron-assisted spin excitation that can exceed in energy and in amplitude a simple excitation among spin states. This excitation, which can be quenched by structural changes in the magnetic molecule, is explained using first-principles calculations that include dynamical electroniccorrelations.es_ES
dc.description.sponsorshipWe thank M. Ternes for providing his fitting program. This work was supported by the Agence Nationale de la Recherche (grants No. ANR-13-BS10-0016, ANR-11-LABX-0058 NIE and ANR-10-LABX-0026 CSC) and by the Agencia Española de Investigación (grants Nos. MAT2016-78293-C6-1-R and MDM-2016-0618). D.-J.C. and N.L. thank the MICINN (project RTI2018-097895-B-C44). M.-L.B. thanks the national computational center CINES and TGCC (GENCI project: A0030807364).es_ES
dc.language.isoenges_ES
dc.publisherNaturees_ES
dc.rightsinfo:eu-repo/semantics/openAccesses_ES
dc.rights.urihttp://creativecommons.org/licenses/by/3.0/es/*
dc.titleVibron-assisted spin excitation in a magnetically anisotropic moleculees_ES
dc.typeinfo:eu-repo/semantics/articlees_ES
dc.rights.holderThis article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/ licenses/by/4.0/.es_ES
dc.rights.holderAtribución 3.0 España*
dc.relation.publisherversionhttps://www.nature.com/articles/s41467-020-15266-0#auth-9es_ES
dc.identifier.doi10.1038/s41467-020-15266-0
dc.departamentoesFísica aplicada Ies_ES
dc.departamentoeuFisika aplikatua Ies_ES


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This article is licensed under a Creative Commons
Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/ licenses/by/4.0/.
Except where otherwise noted, this item's license is described as This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/ licenses/by/4.0/.