Vibron-assisted spin excitation in a magnetically anisotropic molecule
dc.contributor.author | Bachellier, N. | |
dc.contributor.author | Verlhac, B. | |
dc.contributor.author | Garnier, L. | |
dc.contributor.author | Zaldívar, J. | |
dc.contributor.author | Rubio Verdú, Carmen | |
dc.contributor.author | Abufager, P. | |
dc.contributor.author | Ormaza, M. | |
dc.contributor.author | Choi, D. J. | |
dc.contributor.author | Bocquet, M. L. | |
dc.contributor.author | Pascual Chico, José Ignacio ![]() | |
dc.contributor.author | Lorente Palacios, Nicolás | |
dc.contributor.author | Limot, L. | |
dc.date.accessioned | 2020-04-21T08:58:44Z | |
dc.date.available | 2020-04-21T08:58:44Z | |
dc.date.issued | 2020-04 | |
dc.identifier.citation | Nature Communications 11 : (2020) // Article ID 1619 | es_ES |
dc.identifier.issn | 2041-1723 | |
dc.identifier.uri | http://hdl.handle.net/10810/42835 | |
dc.description.abstract | The electrical control and readout of molecular spin states are key for high-density storage. Expectations are that electrically-driven spin and vibrational excitations in a molecule should give rise to new conductance features in the presence of magnetic anisotropy, offering alternative routes to study and, ultimately, manipulate molecular magnetism. Here, we use inelastic electron tunneling spectroscopy to promote and detect the excited spin states of a prototypical molecule with magnetic anisotropy. We demonstrate the existence of a vibron-assisted spin excitation that can exceed in energy and in amplitude a simple excitation among spin states. This excitation, which can be quenched by structural changes in the magnetic molecule, is explained using first-principles calculations that include dynamical electroniccorrelations. | es_ES |
dc.description.sponsorship | We thank M. Ternes for providing his fitting program. This work was supported by the Agence Nationale de la Recherche (grants No. ANR-13-BS10-0016, ANR-11-LABX-0058 NIE and ANR-10-LABX-0026 CSC) and by the Agencia Española de Investigación (grants Nos. MAT2016-78293-C6-1-R and MDM-2016-0618). D.-J.C. and N.L. thank the MICINN (project RTI2018-097895-B-C44). M.-L.B. thanks the national computational center CINES and TGCC (GENCI project: A0030807364). | es_ES |
dc.language.iso | eng | es_ES |
dc.publisher | Nature | es_ES |
dc.rights | info:eu-repo/semantics/openAccess | es_ES |
dc.rights.uri | http://creativecommons.org/licenses/by/3.0/es/ | * |
dc.title | Vibron-assisted spin excitation in a magnetically anisotropic molecule | es_ES |
dc.type | info:eu-repo/semantics/article | es_ES |
dc.rights.holder | This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/ licenses/by/4.0/. | es_ES |
dc.rights.holder | Atribución 3.0 España | * |
dc.relation.publisherversion | https://www.nature.com/articles/s41467-020-15266-0#auth-9 | es_ES |
dc.identifier.doi | 10.1038/s41467-020-15266-0 | |
dc.departamentoes | Física aplicada I | es_ES |
dc.departamentoeu | Fisika aplikatua I | es_ES |
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