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Accessing Chiral Pyrrolodiketopiperazines under Organocatalytic Conditions

dc.contributor.authorDuñabeitia Aizpurúa, Eider
dc.contributor.authorLanda Álvarez, Aitor
dc.contributor.authorLópez Álvarez, Rosa María
dc.contributor.authorPalomo Nicolau, Claudio
dc.date.accessioned2023-05-12T17:51:38Z
dc.date.available2023-05-12T17:51:38Z
dc.date.issued2022-12
dc.identifier.citationOrganic Letters 25(1) : 125-129 (2022)es_ES
dc.identifier.issn1523-7060
dc.identifier.issn1523-7052
dc.identifier.urihttp://hdl.handle.net/10810/61099
dc.description.abstractThe production of chiral pyrrolodiketopiperazines under organocatalytic conditions demonstrates the capacity of bicyclic acylpyrrol lactims to perform as pronucleophiles in direct carbon–carbon bond forming reactions. The good performance of ureidoaminal-derived Brønsted bases in the Michael addition to nitroolefins affords these heterocyclic scaffolds with high skeleton diversity.es_ES
dc.description.sponsorshipFinancial support was provided for the University of the Basque Country UPV/EHU (UFIQOSYC 11/22), the Basque Government (grant IT-1236-19), and Ministerio de Ciencia e Innovation (grant PID2019-109633GB-C21), Spain. E.D. thanks MICINN for a fellowship. We also thank SGiker (UPV/EHU) for providing NMR spectroscopy, HRMS, X-ray, and computational resources.es_ES
dc.language.isoenges_ES
dc.publisherAmerican Chemical Societyes_ES
dc.relationinfo:eu-repo/grantAgreement/MICINN/PID2019-109633GB-C21es_ES
dc.rightsinfo:eu-repo/semantics/openAccesses_ES
dc.rights.urihttp://creativecommons.org/licenses/by/3.0/es/*
dc.titleAccessing Chiral Pyrrolodiketopiperazines under Organocatalytic Conditionses_ES
dc.typeinfo:eu-repo/semantics/articlees_ES
dc.rights.holder© 2022 American Chemical Society. Attribution 4.0 International (CC BY 4.0)es_ES
dc.rights.holderAtribución 3.0 España*
dc.relation.publisherversionhttps://pubs.acs.org/doi/10.1021/acs.orglett.2c03924es_ES
dc.identifier.doi10.1021/acs.orglett.2c03924
dc.departamentoesQuímica orgánica Ies_ES
dc.departamentoeuKimika organikoa Ies_ES


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© 2022 American Chemical Society. Attribution 4.0 International (CC BY 4.0)
Except where otherwise noted, this item's license is described as © 2022 American Chemical Society. Attribution 4.0 International (CC BY 4.0)